报告题目:Preparation of high-efficiency and stable perovskite solar cells
报告人:张博学博士 新加坡国立大学
主持人(邀请人):孙庆、张立军
报告时间:2025年12月22日 14:30-16:00
报告地点:唐敖庆D区429
主办单位:汽车材料教育部重点实验室 在线娱乐城
摘要:Achieving high-performance inverted perovskite solar cells (PSCs) still remains a significant challenge, necessitating innovative approaches in materials selection and manufacturing technique optimization of perovskites. In this work, we unveil a paradigm shift in PSCs optimization. Through a judicious selection from a repertoire of 60 perovskite variants, we identified a composition with exemplary optical, thermal and electrical stability. Employing Bayesian machine learning, we navigated a labyrinth of over 1 billion process conditions, culminating in a record-breaking efficiency within a mere 80 iterations. Finally, the integration of bespoke in situ polymerized ionic molecules allowed us to further augment performance of inverted PSCs, reaching an unparalleled power conversion efficiency of 25.76% (certified at 25.21%). The PSCs retained 94% of the initial efficiency after continuous operation in a nitrogen atmosphere at 65 °C for 1920 hours. This work not only redefines the benchmarks for PSCs but also illuminates the path forward for photovoltaic innovations.
报告人简介:
Boxue Zhang is a Research Fellow at the National University of Singapore. He obtained his PhD degree (2025) in Physical Chemistry from Paris Sciences & Lettres (PSL) University. His research focuses on perovskite solar cells, with particular emphasis on interface engineering, self-assembled monolayers, molecular design, and device stability in single-junction and tandem architectures. He specializes in correlating molecular-level interfacial chemistry with charge transport, defect passivation, and long-term operational stability, aiming to advance both fundamental understanding and practical device performance. He has published as first author and corresponding author in several high-impact journals, including Science, Nature Communications, Energy & Environmental Science, and Angewandte Chemie.